There is much that can be done with simple photocells that would do some of the things that you are asking about. Vactrols are enclosed and have 4 leads, two for the diode and two for the photocell. There effectiveness is based on their response.
You could also use a vactrol for a simple tremolo with the control processor or an LFO from a modular. Simple hook up the LED end to the LFO. You can get cable and 1/4" plugs at Radio Shack or other electronic Herestores on line. Then connect the vactrol LED leads of the vactrol to this. This will cause the LED to pulsate like it does not the Freqbox. You can see this with a vactrol but if you want a visual you can simply buy LEDs (you can get these at Radio Shack too). Then, I believe you may be able to use the mixer of the control processor or some sort of VCA module along with the photo cell either as resistor or combined with voltage sounce, a CV source.
As for the legendary univibe, these did not use vactrol in the sense of single vactrols with four leads but LEDs and photocells.
Here is a good web site:
http://www.lynx.net/~jc/pedalsUnivibe.html
Photocells are very underated musically. For example, you want a cheap therimin (frequency wise). Send an LPF fooger into self oscillation and then plug a photocell (DIY device with plug and photocell) into the frequency. I have done with and with a good flashlight pointing at the cell and you hand in between, you have a cheap therimin.
What should you control? That what I love about foogers. Its up to you. If you use cutoff on an LPF you get a Morley wah (for those technically astute here, yes I know, wahs are bandpass) but something like it. All Morley pedals do is use a photocell to control the frequency of a band pass. The pedal simply translates the movement of the pedal into verticle motion (with gears) to move a cover for the photocell up and down.
If that interests you, consider this. Photo cells come in all sorts of shapes and sizes. Infared, UV, ect. I will let you mind run with that one.
Consider polarized sheets. Create two wheels moving in oppositive directions. A photocell behind them and isolated from light except for the light coming through the filters. You get something that simulates the acceleration and deceleration of Leslie speakers.
By the way, you don’t ever need to open and circut bend you foogers to do this. Just some audio cable, solder, 1/4 plugs and creativity. Sort of what Robert Moog used when he created his wonderful instruments.